Metamodeling methods and their direct methanol fuel cell applications

atmire.migration.oldid1638
dc.contributor.advisorXue, Deyi
dc.contributor.authorYang, Qinwen
dc.date.accessioned2014-02-03T20:29:25Z
dc.date.available2014-03-15T07:00:19Z
dc.date.issued2014-02-03
dc.date.submitted2013en
dc.description.abstractDirect methanol fuel cells (DMFCs) have emerged in recent years as potential power sources for portable electronic devices due to the high energy density of methanol and low power requirements of the portable electronic devices. Fuel cell system modeling plays an important role in the design of DMFC systems. Despite the progress in modeling of DMFCs, most of these models considered only some of the key operating parameters with overly simplified geometric shapes. In addition, since extensive simulations are usually required in design and control of DMFC systems, advanced modeling tools with high computation quality and efficiency are expected. This research focuses on study of adaptive metamodeling methods and applications of these methods in modeling and design of DMFC systems. A semi-empirical model is developed to build the relationships between all important operating parameters and DMFC performance measures. Coefficients of this semi-empirical model are obtained through experiments and data fitting. The semi-empirical model provides a basis to identify the optimal operating parameters of the DMFC system considering different power requirements. In addition, adaptive metamodeling has been employed to describe the electrochemical relationships in a computational fluid dynamics (CFD) based DMFC model to study influences of both geometric parameters and operating parameters on DMFC performance. The CFD-based DMFC model can be used in optimal design of geometric parameters and optimal control of operating parameters. Metamodeling methods, which were initially developed as “surrogates” of the expensive simulation process, can be used to model the relationship between input and output parameters in DMFC systems. Influences of two factors, noise level and initial sample size, on quality of adaptive metamodeling considering different metamodel schemes and test functions are studied in this work. Guidelines have been developed for selection of the proper adaptive metamodeling methods. In addition, a new sampling method namely weighted sequential sampling (WSS) method is introduced in this research to improve the accuracy of adaptive metamodeling considering influences of sample quality measures in both input and output parameter spaces. Quality of the global optimization can be improved based on the metamodel built using the WSS method.en_US
dc.identifier.citationYang, Q. (2014). Metamodeling methods and their direct methanol fuel cell applications (Doctoral thesis, University of Calgary, Calgary, Canada). Retrieved from https://prism.ucalgary.ca. doi:10.11575/PRISM/26887en_US
dc.identifier.doihttp://dx.doi.org/10.11575/PRISM/26887
dc.identifier.urihttp://hdl.handle.net/11023/1364
dc.language.isoeng
dc.publisher.facultyGraduate Studies
dc.publisher.facultySchulich School of Engineering
dc.publisher.institutionUniversity of Calgaryen
dc.publisher.placeCalgaryen
dc.rightsUniversity of Calgary graduate students retain copyright ownership and moral rights for their thesis. You may use this material in any way that is permitted by the Copyright Act or through licensing that has been assigned to the document. For uses that are not allowable under copyright legislation or licensing, you are required to seek permission.
dc.subjectEnergy
dc.subjectEngineering--Mechanical
dc.subject.classificationMetamodelingen_US
dc.subject.classificationSamplingen_US
dc.subject.classificationOptimizationen_US
dc.subject.classificationDirect methanol fuel cellsen_US
dc.titleMetamodeling methods and their direct methanol fuel cell applications
dc.typedoctoral thesis
thesis.degree.disciplineMechanical and Manufacturing Engineering
thesis.degree.grantorUniversity of Calgary
thesis.degree.nameDoctor of Philosophy (PhD)
ucalgary.item.requestcopytrue
Files
Original bundle
Now showing 1 - 1 of 1
Loading...
Thumbnail Image
Name:
ucalgary_2013_yang_qinwen.pdf
Size:
2.23 MB
Format:
Adobe Portable Document Format
Description:
License bundle
Now showing 1 - 1 of 1
Loading...
Thumbnail Image
Name:
license.txt
Size:
2.65 KB
Format:
Item-specific license agreed upon to submission
Description: